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What is the coordination geometry and oxidation state of the metal ion in the active site of the metalloenzyme cytochrome c oxidase responsible for the four-electron reduction of O2 to H2O during cellular respiration?

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ago by (330 points)
Cytochrome c oxidase is a metalloenzyme that plays a crucial role in cellular respiration by catalyzing the reduction of molecular oxygen  O2  to water  H2O . The active site of cytochrome c oxidase contains two metal ions: a high-spin heme a3 iron  Fe  and a copper ion  CuB .The coordination geometry of the heme a3 iron  Fe  is octahedral. The iron is coordinated to a histidine imidazole nitrogen, a porphyrin nitrogen, and an oxygen molecule. The oxygen molecule bridges the iron and copper ions.The coordination geometry of the copper ion  CuB  is square planar. The copper ion is coordinated to three histidine imidazole nitrogens and the bridging oxygen molecule.The oxidation state of the heme a3 iron  Fe  in the active site varies during the catalytic cycle. It can be in the Fe III  or Fe IV  state. The copper ion  CuB  also changes its oxidation state during the catalytic cycle, fluctuating between Cu I  and Cu II .In the fully oxidized state, the heme a3 iron  Fe  is in the Fe IV  state, and the copper ion  CuB  is in the Cu II  state. During the four-electron reduction of O2 to H2O, the oxidation states of the metal ions change to facilitate the transfer of electrons and protons, ultimately returning to their initial oxidation states at the end of the catalytic cycle.
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